Biomass Waste Inspired Highly Porous Carbon for High Performance Lithium/Sulfur Batteries.
Identifieur interne : 001506 ( Main/Exploration ); précédent : 001505; suivant : 001507Biomass Waste Inspired Highly Porous Carbon for High Performance Lithium/Sulfur Batteries.
Auteurs : Yan Zhao [République populaire de Chine] ; Jun Ren [République populaire de Chine] ; Taizhe Tan [République populaire de Chine] ; Moulay-Rachid Babaa [Kazakhstan] ; Zhumabay Bakenov [Kazakhstan] ; Ning Liu [République populaire de Chine] ; Yongguang Zhang [République populaire de Chine]Source :
- Nanomaterials (Basel, Switzerland) [ 2079-4991 ] ; 2017.
Abstract
The synthesis of highly porous carbon (HPC) materials from poplar catkin by KOH chemical activation and hydrothermal carbonization as a conductive additive to a lithium-sulfur cathode is reported. Elemental sulfur was composited with as-prepared HPC through a melt diffusion method to form a S/HPC nanocomposite. Structure and morphology characterization revealed a hierarchically sponge-like structure of HPC with high pore volume (0.62 cm³∙g −1 ) and large specific surface area (1261.7 m²∙g −1 ). When tested in Li/S batteries, the resulting compound demonstrated excellent cycling stability, delivering a second-specific capacity of 1154 mAh∙g −1 as well as presenting 74% retention of value after 100 cycles at 0.1 C. Therefore, the porous structure of HPC plays an important role in enhancing electrochemical properties, which provides conditions for effective charge transfer and effective trapping of soluble polysulfide intermediates, and remarkably improves the electrochemical performance of S/HPC composite cathodes.
DOI: 10.3390/nano7090260
PubMed: 28878149
PubMed Central: PMC5618371
Affiliations:
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first="Taizhe" last="Tan">Taizhe Tan</name><affiliation wicri:level="1"><nlm:affiliation>Synergy Innovation Institute of GDUT, Heyuan 517000, Guangdong, China. taizhetan@gdut.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Synergy Innovation Institute of GDUT, Heyuan 517000, Guangdong</wicri:regionArea><wicri:noRegion>Guangdong</wicri:noRegion></affiliation></author><author><name sortKey="Babaa, Moulay Rachid" sort="Babaa, Moulay Rachid" uniqKey="Babaa M" first="Moulay-Rachid" last="Babaa">Moulay-Rachid Babaa</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Batteries LLC, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. mbabaa@nu.edu.kz.</nlm:affiliation><country xml:lang="fr">Kazakhstan</country><wicri:regionArea>Institute of Batteries LLC, 53 Kabanbay Batyr Avenue, Astana 010000</wicri:regionArea><wicri:noRegion>Astana 010000</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>PI 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Y" first="Yan" last="Zhao">Yan Zhao</name><affiliation wicri:level="1"><nlm:affiliation>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130, China. yanzhao1984@hebut.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130</wicri:regionArea><placeName><settlement type="city">Tianjin</settlement></placeName></affiliation></author><author><name sortKey="Ren, Jun" sort="Ren, Jun" uniqKey="Ren J" first="Jun" last="Ren">Jun Ren</name><affiliation wicri:level="1"><nlm:affiliation>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130, China. 201631804046@stu.hebut.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130</wicri:regionArea><placeName><settlement type="city">Tianjin</settlement></placeName></affiliation></author><author><name sortKey="Tan, Taizhe" sort="Tan, Taizhe" uniqKey="Tan T" first="Taizhe" last="Tan">Taizhe Tan</name><affiliation wicri:level="1"><nlm:affiliation>Synergy Innovation Institute of GDUT, Heyuan 517000, Guangdong, China. taizhetan@gdut.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Synergy Innovation Institute of GDUT, Heyuan 517000, Guangdong</wicri:regionArea><wicri:noRegion>Guangdong</wicri:noRegion></affiliation></author><author><name sortKey="Babaa, Moulay Rachid" sort="Babaa, Moulay Rachid" uniqKey="Babaa M" first="Moulay-Rachid" last="Babaa">Moulay-Rachid Babaa</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Batteries LLC, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. mbabaa@nu.edu.kz.</nlm:affiliation><country xml:lang="fr">Kazakhstan</country><wicri:regionArea>Institute of Batteries LLC, 53 Kabanbay Batyr Avenue, Astana 010000</wicri:regionArea><wicri:noRegion>Astana 010000</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>PI National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. mbabaa@nu.edu.kz.</nlm:affiliation><country xml:lang="fr">Kazakhstan</country><wicri:regionArea>PI National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000</wicri:regionArea><wicri:noRegion>Astana 010000</wicri:noRegion></affiliation></author><author><name sortKey="Bakenov, Zhumabay" sort="Bakenov, Zhumabay" uniqKey="Bakenov Z" first="Zhumabay" last="Bakenov">Zhumabay Bakenov</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Batteries LLC, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. zbakenov@nu.edu.kz.</nlm:affiliation><country xml:lang="fr">Kazakhstan</country><wicri:regionArea>Institute of Batteries LLC, 53 Kabanbay Batyr Avenue, Astana 010000</wicri:regionArea><wicri:noRegion>Astana 010000</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>PI National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. zbakenov@nu.edu.kz.</nlm:affiliation><country xml:lang="fr">Kazakhstan</country><wicri:regionArea>PI National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000</wicri:regionArea><wicri:noRegion>Astana 010000</wicri:noRegion></affiliation></author><author><name sortKey="Liu, Ning" sort="Liu, Ning" uniqKey="Liu N" first="Ning" last="Liu">Ning Liu</name><affiliation wicri:level="1"><nlm:affiliation>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130, China. ningliu1985@hebut.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130</wicri:regionArea><placeName><settlement type="city">Tianjin</settlement></placeName></affiliation></author><author><name sortKey="Zhang, Yongguang" sort="Zhang, Yongguang" uniqKey="Zhang Y" first="Yongguang" last="Zhang">Yongguang Zhang</name><affiliation wicri:level="1"><nlm:affiliation>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130, China. yongguangzhang@hebut.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130</wicri:regionArea><placeName><settlement type="city">Tianjin</settlement></placeName></affiliation></author></analytic><series><title level="j">Nanomaterials (Basel, Switzerland)</title><idno type="ISSN">2079-4991</idno><imprint><date when="2017" type="published">2017</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The synthesis of highly porous carbon (HPC) materials from poplar catkin by KOH chemical activation and hydrothermal carbonization as a conductive additive to a lithium-sulfur cathode is reported. Elemental sulfur was composited with as-prepared HPC through a melt diffusion method to form a S/HPC nanocomposite. Structure and morphology characterization revealed a hierarchically sponge-like structure of HPC with high pore volume (0.62 cm³∙g <sup>−1</sup> ) and large specific surface area (1261.7 m²∙g <sup>−1</sup> ). When tested in Li/S batteries, the resulting compound demonstrated excellent cycling stability, delivering a second-specific capacity of 1154 mAh∙g <sup>−1</sup> as well as presenting 74% retention of value after 100 cycles at 0.1 C. Therefore, the porous structure of HPC plays an important role in enhancing electrochemical properties, which provides conditions for effective charge transfer and effective trapping of soluble polysulfide intermediates, and remarkably improves the electrochemical performance of S/HPC composite cathodes.</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">28878149</PMID><DateRevised><Year>2020</Year><Month>09</Month><Day>29</Day></DateRevised><Article PubModel="Electronic"><Journal><ISSN IssnType="Print">2079-4991</ISSN><JournalIssue CitedMedium="Print"><Volume>7</Volume><Issue>9</Issue><PubDate><Year>2017</Year><Month>Sep</Month><Day>06</Day></PubDate></JournalIssue><Title>Nanomaterials (Basel, Switzerland)</Title><ISOAbbreviation>Nanomaterials (Basel)</ISOAbbreviation></Journal><ArticleTitle>Biomass Waste Inspired Highly Porous Carbon for High Performance Lithium/Sulfur Batteries.</ArticleTitle><ELocationID EIdType="pii" ValidYN="Y">E260</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.3390/nano7090260</ELocationID><Abstract><AbstractText>The synthesis of highly porous carbon (HPC) materials from poplar catkin by KOH chemical activation and hydrothermal carbonization as a conductive additive to a lithium-sulfur cathode is reported. Elemental sulfur was composited with as-prepared HPC through a melt diffusion method to form a S/HPC nanocomposite. Structure and morphology characterization revealed a hierarchically sponge-like structure of HPC with high pore volume (0.62 cm³∙g <sup>−1</sup> ) and large specific surface area (1261.7 m²∙g <sup>−1</sup> ). When tested in Li/S batteries, the resulting compound demonstrated excellent cycling stability, delivering a second-specific capacity of 1154 mAh∙g <sup>−1</sup> as well as presenting 74% retention of value after 100 cycles at 0.1 C. Therefore, the porous structure of HPC plays an important role in enhancing electrochemical properties, which provides conditions for effective charge transfer and effective trapping of soluble polysulfide intermediates, and remarkably improves the electrochemical performance of S/HPC composite cathodes.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Zhao</LastName><ForeName>Yan</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130, China. yanzhao1984@hebut.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Ren</LastName><ForeName>Jun</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130, China. 201631804046@stu.hebut.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Tan</LastName><ForeName>Taizhe</ForeName><Initials>T</Initials><AffiliationInfo><Affiliation>Synergy Innovation Institute of GDUT, Heyuan 517000, Guangdong, China. taizhetan@gdut.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Babaa</LastName><ForeName>Moulay-Rachid</ForeName><Initials>MR</Initials><AffiliationInfo><Affiliation>Institute of Batteries LLC, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. mbabaa@nu.edu.kz.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>PI National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. mbabaa@nu.edu.kz.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Bakenov</LastName><ForeName>Zhumabay</ForeName><Initials>Z</Initials><AffiliationInfo><Affiliation>Institute of Batteries LLC, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. zbakenov@nu.edu.kz.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>PI National Laboratory Astana, School of Engineering, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan. zbakenov@nu.edu.kz.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Liu</LastName><ForeName>Ning</ForeName><Initials>N</Initials><AffiliationInfo><Affiliation>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130, China. ningliu1985@hebut.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Yongguang</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, Hebei University of Technology, Tianjin 300130, China. yongguangzhang@hebut.edu.cn.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2017</Year><Month>09</Month><Day>06</Day></ArticleDate></Article><MedlineJournalInfo><Country>Switzerland</Country><MedlineTA>Nanomaterials (Basel)</MedlineTA><NlmUniqueID>101610216</NlmUniqueID><ISSNLinking>2079-4991</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">cathode</Keyword><Keyword MajorTopicYN="N">lithium/sulfur battery</Keyword><Keyword MajorTopicYN="N">poplar catkin</Keyword><Keyword MajorTopicYN="N">sulfur/highly porous carbon composite</Keyword></KeywordList><CoiStatement>The authors declare no conflict of interest.</CoiStatement></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2017</Year><Month>07</Month><Day>30</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2017</Year><Month>08</Month><Day>27</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2017</Year><Month>09</Month><Day>01</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2017</Year><Month>9</Month><Day>8</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2017</Year><Month>9</Month><Day>8</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2017</Year><Month>9</Month><Day>8</Day><Hour>6</Hour><Minute>1</Minute></PubMedPubDate></History><PublicationStatus>epublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">28878149</ArticleId><ArticleId IdType="pii">nano7090260</ArticleId><ArticleId IdType="doi">10.3390/nano7090260</ArticleId><ArticleId IdType="pmc">PMC5618371</ArticleId></ArticleIdList><ReferenceList><Reference><Citation>Chem Rev. 2014 Dec 10;114(23):11751-87</Citation><ArticleIdList><ArticleId IdType="pubmed">25026475</ArticleId></ArticleIdList></Reference><Reference><Citation>Acc Chem Res. 2015 Nov 17;48(11):2947-56</Citation><ArticleIdList><ArticleId IdType="pubmed">26496667</ArticleId></ArticleIdList></Reference><Reference><Citation>J Am Chem Soc. 2012 Nov 14;134(45):18510-3</Citation><ArticleIdList><ArticleId IdType="pubmed">23101502</ArticleId></ArticleIdList></Reference><Reference><Citation>Nat Mater. 2011 Dec 15;11(1):19-29</Citation><ArticleIdList><ArticleId 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Zhang</name></country><country name="Kazakhstan"><noRegion><name sortKey="Babaa, Moulay Rachid" sort="Babaa, Moulay Rachid" uniqKey="Babaa M" first="Moulay-Rachid" last="Babaa">Moulay-Rachid Babaa</name></noRegion><name sortKey="Babaa, Moulay Rachid" sort="Babaa, Moulay Rachid" uniqKey="Babaa M" first="Moulay-Rachid" last="Babaa">Moulay-Rachid Babaa</name><name sortKey="Bakenov, Zhumabay" sort="Bakenov, Zhumabay" uniqKey="Bakenov Z" first="Zhumabay" last="Bakenov">Zhumabay Bakenov</name><name sortKey="Bakenov, Zhumabay" sort="Bakenov, Zhumabay" uniqKey="Bakenov Z" first="Zhumabay" last="Bakenov">Zhumabay Bakenov</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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